Note
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ISOTOPE
¶
Generation of the FORCE matrix is very time-consuming,
and in isotopic substitution studies several vibrational calculations
may be needed. To allow the frequencies to be calculated from the
(constant) force matrix, ISOTOPE
is used. When a FORCE
calculation is completed, ISOTOPE
will cause the force matrix to be
stored, regardless of whether or not any intervening restarts have been
made. To re-calculate the frequencies, etc., starting at the end of the
force matrix calculation, specify RESTART
.
The two keywords RESTART
and ISOTOPE
can be used together. For
example, if a normal FORCE
calculation runs for a long time, the
user may want to divide it up into stages and save the final force
matrix. Once ISOTOPE
has been used, it does not need to be used on
subsequent RESTART
runs. ISOTOPE
can also be used with FORCE
to set up a RESTART
file for an IRC=n
calculation.